One of the most intriguing combinations is Harley Quinn and Alice Cullen. Harley's chaotic and unpredictable nature paired with Alice's calm and prescient abilities would create a really interesting dynamic. They could either be at odds or find a strange kind of friendship. Another good combination is Deadshot and Edward Cullen. Deadshot's sharpshooting skills and his more jaded view of the world contrasted with Edward's brooding and his vampiric powers would make for some great scenes.
One interesting pairing could be Edward and Deadshot. Edward's ability to read minds could be really useful in helping Deadshot with his aiming. Deadshot, on the other hand, could teach Edward about human combat techniques that the vampires might not be familiar with.
A cool plot would involve some of the Suicide Squad members getting turned into vampires. Imagine Deadshot with vampire powers, his already excellent shooting skills enhanced by superhuman speed and strength. The Twilight characters would be divided on whether to help the Squad or destroy them. Bella could be intrigued by the 'human - like' yet different nature of the Squad members and try to understand their world.
I think Thor and Carlisle would be really interesting. Thor is a god with all his power and Carlisle is an old - school vampire with a strong moral code. They could have some deep conversations about life, death, and power. And then there's Jacob and Bruce Banner. Jacob's hot - headedness and Bruce's struggle with his inner Hulk could lead to some intense situations. Maybe Jacob could help Bruce control the Hulk in some way, or they could get into a big fight that the others have to break up.
Sasuke and a fox demon with a similar past of loss. Sasuke has his own dark past with the Uchiha clan's massacre. A fox demon who has lost their family or pack could bond with Sasuke over their shared experiences. They might even develop a unique fighting style together, combining Sasuke's Sharingan - enhanced jutsu with the fox demon's special abilities.
Naruto and Inuyasha themselves would be a very intriguing combination. Naruto's positive attitude and never - give - up spirit combined with Inuyasha's rough - around - the - edges but strong - willed personality would create a lot of interesting interactions. They could start off not liking each other but gradually become friends as they face challenges together.
One intriguing combination would be Hermione and Neytiri. Hermione's thirst for knowledge and Neytiri's connection to Pandora's nature could lead to some great interactions. Hermione could learn from Neytiri about the unique flora and fauna of Pandora, and Neytiri could be fascinated by Hermione's magic and her ability to study and understand complex things.
Deadpool, without a doubt. His crazy antics, fourth - wall - breaking, and unpredictable nature would add a whole new level of chaos to the already volatile Suicide Squad. He would constantly be making jokes, getting into fights with the other members just for the fun of it, and finding unique ways to solve problems that the more traditional Squad members wouldn't think of.
One of the most interesting plot twists could be when Harley realizes that Joker's love for her is just a part of his game. In many Suicide Squad interpretations, Harley is blindly in love with Joker. But if she discovers his true nature, it flips the whole dynamic. It makes her question her loyalty and could lead to her breaking free from his control and becoming a more independent character within the fanfic.
One interesting crossover could be a scenario where the vampires from Twilight interact with the super - villains of Suicide Squad. For example, the vampires' superhuman abilities might be pitted against the Squad's unique skills and weaponry. It could create some really intense battle scenes.
One popular theme is redemption. In Twilight Suicide Squad fanfiction, characters who are often seen as villains in their original stories get a chance to redeem themselves. For example, a member of the Suicide Squad might find a new purpose that goes against their previous life of crime. Another theme could be the clash of different universes. Since it combines Twilight and Suicide Squad, there can be interesting interactions between the supernatural elements of Twilight, like vampires and werewolves, and the anti - hero nature of the Suicide Squad. Also, friendship and loyalty within the squad in the context of this strange new crossover world can be a theme, as they have to rely on each other despite their differences.